A similar problem is A018805, where a(n) is the number of coprime pairs
(x, y) with 1 <= x,y <= n.  I found the recursion
 
a(n) = n^2 - SUM(j=2..n; a(floor(n/j)))
 
This recusion is gotten by noticing that the number of pairs (x,y) with
gcd(x,y) = j, 1 <= x,y <= n, is just a(floor(n/j)).  So a(n) is gotten
by taking all n^2 pairs, and subtracting out those whose gcd's fall
between 2 and n.
 
With clever programming, this identity is the basis for a fairly quick
algorithm for a(n), much faster than the obvious SUM(j=1..n; phi(j)).
 
I was hoping something similar might be done with A027424.  For example,
observe that the number of distinct even entries in the n x n
multiplication table is just the number of distinct entries in the
n x floor(n/2) multiplication table, analogously for entries divisible
by other primes.